Dust and Cables: Addressing Major Background Concerns in Rare-Event Ultralow Background Physics Experiments

14 Feb 2024, 19:20
10m
ES635 (KMI Science Symposia)

ES635

KMI Science Symposia

Speaker

Dr Isaac Arnquist (Pacific Northwest National Laboratory)

Description

Dust particulate fallout on materials in use for rare-event searches is a concerning source of radioactive backgrounds due to the presence of the naturally occurring radionuclides. Much effort is dedicated to understanding backgrounds from dust and evaluating mitigation procedures. In this work, an ICP-MS based methodology is presented that demonstrates a direct determination of fallout rates of radionuclides and stable isotopes of interest from dust particulate at the SNOLAB facility. This work validates the mitigation procedures in place at SNOLAB and informs dust backgrounds during laboratory activities. Fallout rates of major constituents of the local rock were measured two to three orders of magnitude lower in the clean experimental areas compared to non-clean transition areas from the mine to the laboratory. Increased radiocontaminant fallout rates were measured in clean experimental areas during activities generating particulate. Flexible printed cables and circuitry based on copper-polyimide materials are widely used in experiments looking for rare events due to their unique electrical and mechanical characteristics. However, past studies have found copper-polyimide flexible cables to contain 400-4700 pg 238U/g, 16-3700 pg 232Th/g, and 170-2100 ng natK/g, which can be a significant source of radioactive background for many current and next-generation ultralow background detectors. This work presents a comprehensive investigation into the fabrication process of copper-polyimide flexible cables and the development of custom low radioactivity cables for use in rare-event physics applications. Radiopure material alternatives were identified, and cleaner production processes and treatments were developed to significantly reduce the imparted contamination. Through the newly developed radiopure fabrication process, fully-functioning cables were produced with radiocontaminant concentrations of 20-31 pg 238U/g, 12-13 pg 232Th/g, and 40-550 ng natK/g, which is significantly cleaner than cables from previous work and sufficiently radiopure for current and next-generation detectors. This approach, employing witness samples to investigate each step of the fabrication process, can hopefully serve as a template for investigating radiocontaminants in other material production processes.

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